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In this work, an atmospheric nanoparticle model with 59 wt% SA was constructed, and the heterogeneous reactions of DMA/ammonia with SA in the air-nanoparticle interface in addition to inside the bulk nanoparticle have been comparably investigated with theoretical methods. The results revealed that the interface reaction mechanism of DMA to promote atmospheric nanoparticle development is totally different from that of ammonia.

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